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Wakaida, Ikuo; Oba, Hironori; Miyabe, Masabumi; Akaoka, Katsuaki; Oba, Masaki; Tamura, Koji; Saeki, Morihisa
Kogaku, 48(1), p.13 - 20, 2019/01
By Laser Induced Breakdown Spectroscopy and by related resonance spectroscopy, elemental and isotope analysis of Uranium and Plutonium for nuclear fuel materials and in-situ remote analysis under strong radiation condition for melt downed nuclear fuel debris at damaged core in "Fukushima Daiichi Nuclear Power Station", are introduced and performed as one of the application in atomic energy research field.
Miyabe, Masabumi; Oda, Koichi*; Oba, Masaki; Kato, Masaaki; Wakaida, Ikuo; Watanabe, Kazuo
JAERI-Tech 2004-064, 33 Pages, 2004/10
JAERI-Tech-2004-064.pdf:1.89MB
In nuclear waste materials there are various radionuclides to which standard analytical techniques are difficult to be applied. We are developing an analytical technique where such nuclides are analyzed using multi-step resonance ionization mass spectrometry. In this study, we have developed an external cavity diode laser applicable to the analysis. The wavelength and output power dependence on injection current and temperature were investigated for various types of laser diodes. Based on the data, we have obtained a suitable condition to operate the ECDL in stable single-mode oscillation, so that a continuous scanning range of about 100 GHz was realized. Additionaly, to evaluate the bandwidth of the developed ECDL, we have performed Doppler-free spectroscopy. The reasonable agreement of the measured isotope shift and HFS splitting with the reported values demonstrated that the developed ECDL is applicable to a precise laser spectroscopy as well as a laser trace analysis.
Yokoya, Akinari; Takakura, Kaoru*; Watanabe, Ritsuko; Akamatsu, Ken*; Ito, Takashi*
Radiation Research, 162(4), p.469 - 473, 2004/10
Times Cited Count：3 Percentile：10.06(Biology)X-ray absorption spectra from single crystals of 5-Bromouracil were measured with the transmission mode in the energy range from 13.41 to 13.50 keV using the linearly polarized synchrotron radiation (SR). A characteristic resonance structure, consisting of four peaks, was recognized in the spectra in the Br K-edge region. The intensities of these peaks were strongly dependent on the crystal rotation about the normal of the crystal b-c plane, which was set perpendicular to the X-ray beam direction. (SR X-rays are polarized in the horizontal plane.) Molecular orbital calculations indicate that these resonance peaks are associated with the transitions from the 1s electron of Br to the Br-C molecular antibonding orbitals and to a shape resonance. The observed anisotropy of each photoabsorption peak might originate from the angular dependences of these molecular orbitals.
Okumura, Keisuke; *;
JAERI-Data/Code 96-015, 445 Pages, 1996/03
JAERI-Data-Code-96-015.pdf:12.94MB
no abstracts in English
Kugo, Teruhiko; ; *
Journal of Nuclear Science and Technology, 27(9), p.870 - 874, 1990/09
no abstracts in English
JAERI-M 85-034, 206 Pages, 1985/03
no abstracts in English
; ; *
Journal of Nuclear Science and Technology, 22(1), p.16 - 27, 1985/00
Times Cited Count：11 Percentile：78.53(Nuclear Science & Technology)no abstracts in English
*; ; ;
JAERI-M 83-176, 121 Pages, 1983/11
no abstracts in English
;
Nuclear Science and Engineering, 31, p.388 - 395, 1968/00
Times Cited Count：11no abstracts in English
Nuclear Science and Engineering, 32, p.423 - 426, 1968/00
no abstracts in English
UTone, Tatsuzo; ;
Journal of Nuclear Science and Technology, 4(12), p.601 - 606, 1967/00
Times Cited Count：2no abstracts in English
DyP.K.Tseng*; ; ;
Journal of the Physical Society of Japan, 16(9), p.1790 - 1790, 1961/00
Times Cited Count：1no abstracts in English
Wakaida, Ikuo; Oba, Hironori; Akaoka, Katsuaki; Miyabe, Masabumi; Oba, Masaki; Ito, Chikara; Saeki, Morihisa; Kato, Masaaki
no journal, ,
In nuclear engineering, especially for the decommissioning of severe accident atomic power plant, development of quick, easy, non-contact, no-preparation, direct, remote, onsite and in-situ analysis of nuclear fuel materials which has very complex and large amount of optical emission lines will be indispensable. In these R&D, it may be important how we realize high sensitivity and high resolution spectroscopy and perform the identification of the specific element among a large number of emission spectra. Various kind of technique, such as Double-pulse LIBS and Microwave assisted LIBS for multiply the emission intensity, high resolution LIBS by ultra-high resolution spectrometer or Laser Ablation Resonance Absorption Spectroscopy for isotope analysis, Ultra-thin Liquid flow LIBS for liquid phase application and LIBS based on radiation resistant optical fiber for onsite/in-situ monitoring of melt downed nuclear fuel debris, will have been under investigation. Japan Atomic Energy Agency has opened the new research center "Collaborative Laboratories for Advanced Decommissioning Science", and laser based spectroscopy will be restarted as one of the basic projects.
Kai, Tetsuya; Matsumoto, Yoshihiro*; Parker, J. D.*; Segawa, Mariko; Shinohara, Takenao; Hiroi, Kosuke; Su, Y. H.; Zhang, S.*; Hayashida, Hirotoshi*; Oikawa, Kenichi; et al.
no journal, ,
Wakaida, Ikuo; Akaoka, Katsuaki; Miyabe, Masabumi; Oba, Hironori; Saeki, Morihisa; Oba, Masaki; Ito, Chikara; Kato, Masaaki
no journal, ,
Laser Induced Breakdown Spectroscopy (LIBS) for elemental analysis and Laser Ablation Resonance Absorption Spectroscopy (LARAS) for isotope analysis have been developed as an analytical technique for Low-decontaminated MOX fuel with fissionable Miner Actinide elements (MA) and as for one of the diagnostic tool of nuclear fuel debris and polluted materials in the decommissioning of the severe accident nuclear power station. Specialized glove box with auto and remote arraignment system for LIBS and LARAS was constructed, and the detection limit of Pu in MOX to be several 1000 ppm and some hyper fine structures of 
Pu were demonstrated. For the diagnostic tool in the decommissioning of damaged core, optical fiber based portable LIBS probe made by radiation resistant optical fiber is under construction, and just now, some specific spectra from the simulated sample of molten debris made by sintered oxide of Zr and U is successfully observed under water condition or strong radiation field.
Wakaida, Ikuo; Oba, Hironori; Miyabe, Masabumi; Akaoka, Katsuaki; Tamura, Koji; Saeki, Morihisa; Oba, Masaki; Shibata, Takuya; Ikeda, Yuji*; Sakka, Tetsuo*; et al.
no journal, ,
